Rehder Gregor

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Rehder
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Gregor
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  • Article
    Ideas and perspectives: a strategic assessment of methane and nitrous oxide measurements in the marine environment
    (European Geosciences Union, 2020-11-26) Wilson, Samuel T. ; Al-Haj, Alia N. ; Bourbonnais, Annie ; Frey, Claudia ; Fulweiler, Robinson W. ; Kessler, John D. ; Marchant, Hannah K. ; Milucka, Jana ; Ray, Nicholas E. ; Suntharalingam, Parvadha ; Thornton, Brett F. ; Upstill-Goddard, Robert C. ; Weber, Thomas S. ; Arévalo-Martínez, Damian L. ; Bange, Hermann W. ; Benway, Heather M. ; Bianchi, Daniele ; Borges, Alberto V. ; Chang, Bonnie X. ; Crill, Patrick M. ; del Valle, Daniela A. ; Farías, Laura ; Joye, Samantha B. ; Kock, Annette ; Labidi, Jabrane ; Manning, Cara C. ; Pohlman, John W. ; Rehder, Gregor ; Sparrow, Katy J. ; Tortell, Philippe D. ; Treude, Tina ; Valentine, David L. ; Ward, Bess B. ; Yang, Simon ; Yurganov, Leonid N.
    In the current era of rapid climate change, accurate characterization of climate-relevant gas dynamics – namely production, consumption, and net emissions – is required for all biomes, especially those ecosystems most susceptible to the impact of change. Marine environments include regions that act as net sources or sinks for numerous climate-active trace gases including methane (CH4) and nitrous oxide (N2O). The temporal and spatial distributions of CH4 and N2O are controlled by the interaction of complex biogeochemical and physical processes. To evaluate and quantify how these mechanisms affect marine CH4 and N2O cycling requires a combination of traditional scientific disciplines including oceanography, microbiology, and numerical modeling. Fundamental to these efforts is ensuring that the datasets produced by independent scientists are comparable and interoperable. Equally critical is transparent communication within the research community about the technical improvements required to increase our collective understanding of marine CH4 and N2O. A workshop sponsored by Ocean Carbon and Biogeochemistry (OCB) was organized to enhance dialogue and collaborations pertaining to marine CH4 and N2O. Here, we summarize the outcomes from the workshop to describe the challenges and opportunities for near-future CH4 and N2O research in the marine environment.
  • Article
    Global carbon budget 2017
    (Copernicus Publications on behalf of the European Geosciences Union, 2018-03-12) Le Quere, Corinne ; Andrew, Robbie M. ; Friedlingstein, Pierre ; Sitch, Stephen ; Pongratz, Julia ; Manning, Andrew C. ; Korsbakken, Jan Ivar ; Peters, Glen P. ; Canadell, Josep G. ; Jackson, Robert B. ; Boden, Thomas A. ; Tans, Pieter P. ; Andrews, Oliver D. ; Arora, Vivek K. ; Bakker, Dorothee ; Barbero, Leticia ; Becker, Meike ; Betts, Richard A. ; Bopp, Laurent ; Chevallier, Frédéric ; Chini, Louise Parsons ; Ciais, Philippe ; Cosca, Catherine E. ; Cross, Jessica N. ; Currie, Kim I. ; Gasser, Thomas ; Harris, Ian ; Hauck, Judith ; Haverd, Vanessa ; Houghton, Richard A. ; Hunt, Christopher W. ; Hurtt, George ; Ilyina, Tatiana ; Jain, Atul K. ; Kato, Etsushi ; Kautz, Markus ; Keeling, Ralph F. ; Klein Goldewijk, Kees ; Körtzinger, Arne ; Landschützer, Peter ; Lefèvre, Nathalie ; Lenton, Andrew ; Lienert, Sebastian ; Lima, Ivan D. ; Lombardozzi, Danica ; Metzl, Nicolas ; Millero, Frank J. ; Monteiro, Pedro M. S. ; Munro, David R. ; Nabel, Julia E. M. S. ; Nakaoka, Shin-ichiro ; Nojiri, Yukihiro ; Padin, X. Antonio ; Peregon, Anna ; Pfeil, Benjamin ; Pierrot, Denis ; Poulter, Benjamin ; Rehder, Gregor ; Reimer, Janet ; Rödenbeck, Christian ; Schwinger, Jorg ; Séférian, Roland ; Skjelvan, Ingunn ; Stocker, Benjamin D. ; Tian, Hanqin ; Tilbrook, Bronte ; Tubiello, Francesco N. ; van der Laan-Luijkx, Ingrid T. ; van der Werf, Guido R. ; van Heuven, Steven ; Viovy, Nicolas ; Vuichard, Nicolas ; Walker, Anthony P. ; Watson, Andrew J. ; Wiltshire, Andrew J. ; Zaehle, Sonke ; Zhu, Dan
    Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere – the "global carbon budget" – is important to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. CO2 emissions from fossil fuels and industry (EFF) are based on energy statistics and cement production data, respectively, while emissions from land-use change (ELUC), mainly deforestation, are based on land-cover change data and bookkeeping models. The global atmospheric CO2 concentration is measured directly and its rate of growth (GATM) is computed from the annual changes in concentration. The ocean CO2 sink (SOCEAN) and terrestrial CO2 sink (SLAND) are estimated with global process models constrained by observations. The resulting carbon budget imbalance (BIM), the difference between the estimated total emissions and the estimated changes in the atmosphere, ocean, and terrestrial biosphere, is a measure of imperfect data and understanding of the contemporary carbon cycle. All uncertainties are reported as ±1σ. For the last decade available (2007–2016), EFF was 9.4 ± 0.5 GtC yr−1, ELUC 1.3 ± 0.7 GtC yr−1, GATM 4.7 ± 0.1 GtC yr−1, SOCEAN 2.4 ± 0.5 GtC yr−1, and SLAND 3.0 ± 0.8 GtC yr−1, with a budget imbalance BIM of 0.6 GtC yr−1 indicating overestimated emissions and/or underestimated sinks. For year 2016 alone, the growth in EFF was approximately zero and emissions remained at 9.9 ± 0.5 GtC yr−1. Also for 2016, ELUC was 1.3 ± 0.7 GtC yr−1, GATM was 6.1 ± 0.2 GtC yr−1, SOCEAN was 2.6 ± 0.5 GtC yr−1, and SLAND was 2.7 ± 1.0 GtC yr−1, with a small BIM of −0.3 GtC. GATM continued to be higher in 2016 compared to the past decade (2007–2016), reflecting in part the high fossil emissions and the small SLAND consistent with El Niño conditions. The global atmospheric CO2 concentration reached 402.8 ± 0.1 ppm averaged over 2016. For 2017, preliminary data for the first 6–9 months indicate a renewed growth in EFF of +2.0 % (range of 0.8 to 3.0 %) based on national emissions projections for China, USA, and India, and projections of gross domestic product (GDP) corrected for recent changes in the carbon intensity of the economy for the rest of the world. This living data update documents changes in the methods and data sets used in this new global carbon budget compared with previous publications of this data set (Le Quéré et al., 2016, 2015b, a, 2014, 2013). All results presented here can be downloaded from https://doi.org/10.18160/GCP-2017 (GCP, 2017).
  • Article
    An intercomparison of oceanic methane and nitrous oxide measurements
    (Copernicus Publications on behalf of the European Geosciences Union, 2018-10-05) Wilson, Samuel T. ; Bange, Hermann W. ; Arévalo-Martínez, Damian L. ; Barnes, Jonathan ; Borges, Alberto V. ; Brown, Ian ; Bullister, John L. ; Burgos, Macarena ; Capelle, David W. ; Casso, Michael A. ; de la Paz, Mercedes ; Farías, Laura ; Fenwick, Lindsay ; Ferrón, Sara ; Garcia, Gerardo ; Glockzin, Michael ; Karl, David M. ; Kock, Annette ; Laperriere, Sarah ; Law, Cliff S. ; Manning, Cara C. ; Marriner, Andrew ; Myllykangas, Jukka-Pekka ; Pohlman, John W. ; Rees, Andrew P. ; Santoro, Alyson E. ; Tortell, Philippe D. ; Upstill-Goddard, Robert C. ; Wisegarver, David P. ; Zhang, Gui-Ling ; Rehder, Gregor
    Large-scale climatic forcing is impacting oceanic biogeochemical cycles and is expected to influence the water-column distribution of trace gases, including methane and nitrous oxide. Our ability as a scientific community to evaluate changes in the water-column inventories of methane and nitrous oxide depends largely on our capacity to obtain robust and accurate concentration measurements that can be validated across different laboratory groups. This study represents the first formal international intercomparison of oceanic methane and nitrous oxide measurements whereby participating laboratories received batches of seawater samples from the subtropical Pacific Ocean and the Baltic Sea. Additionally, compressed gas standards from the same calibration scale were distributed to the majority of participating laboratories to improve the analytical accuracy of the gas measurements. The computations used by each laboratory to derive the dissolved gas concentrations were also evaluated for inconsistencies (e.g., pressure and temperature corrections, solubility constants). The results from the intercomparison and intercalibration provided invaluable insights into methane and nitrous oxide measurements. It was observed that analyses of seawater samples with the lowest concentrations of methane and nitrous oxide had the lowest precisions. In comparison, while the analytical precision for samples with the highest concentrations of trace gases was better, the variability between the different laboratories was higher: 36% for methane and 27% for nitrous oxide. In addition, the comparison of different batches of seawater samples with methane and nitrous oxide concentrations that ranged over an order of magnitude revealed the ramifications of different calibration procedures for each trace gas. Finally, this study builds upon the intercomparison results to develop recommendations for improving oceanic methane and nitrous oxide measurements, with the aim of precluding future analytical discrepancies between laboratories.
  • Article
    Global Carbon Budget 2015
    (Copernicus Publications, 2015-12-07) Le Quere, Corinne ; Moriarty, Roisin ; Andrew, Robbie M. ; Canadell, Josep G. ; Sitch, Stephen ; Korsbakken, Jan Ivar ; Friedlingstein, Pierre ; Peters, Glen P. ; Andres, Robert J. ; Boden, Thomas A. ; Houghton, Richard A. ; House, Jo I. ; Keeling, Ralph F. ; Tans, Pieter P. ; Arneth, Almut ; Bakker, Dorothee C. E. ; Barbero, Leticia ; Bopp, Laurent ; Chang, J. ; Chevallier, Frédéric ; Chini, Louise Parsons ; Ciais, Philippe ; Fader, Marianela ; Feely, Richard A. ; Gkritzalis, Thanos ; Harris, Ian ; Hauck, Judith ; Ilyina, Tatiana ; Jain, Atul K. ; Kato, Etsushi ; Kitidis, Vassilis ; Klein Goldewijk, Kees ; Koven, Charles ; Landschutzer, Peter ; Lauvset, Siv K. ; Lefevre, N. ; Lenton, Andrew ; Lima, Ivan D. ; Metzl, Nicolas ; Millero, Frank J. ; Munro, David R. ; Murata, Akihiko ; Nabel, Julia E. M. S. ; Nakaoka, Shin-ichiro ; Nojiri, Yukihiro ; O'Brien, Kevin ; Olsen, Are ; Ono, Tsuneo ; Perez, Fiz F. ; Pfeil, Benjamin ; Pierrot, Denis ; Poulter, Benjamin ; Rehder, Gregor ; Rodenbeck, C. ; Saito, Shu ; Schuster, Ute ; Schwinger, Jorg ; Seferian, Roland ; Steinhoff, Tobias ; Stocker, Benjamin D. ; Sutton, Adrienne J. ; Takahashi, Taro ; Tilbrook, Bronte ; van der Laan-Luijkx, I. T. ; van der Werf, Guido R. ; van Heuven, Steven ; Vandemark, Douglas ; Viovy, Nicolas ; Wiltshire, Andrew J. ; Zaehle, Sonke ; Zeng, Ning
    Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere is important to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe data sets and a methodology to quantify all major components of the global carbon budget, including their uncertainties, based on the combination of a range of data, algorithms, statistics, and model estimates and their interpretation by a broad scientific community. We discuss changes compared to previous estimates as well as consistency within and among components, alongside methodology and data limitations. CO2 emissions from fossil fuels and industry (EFF) are based on energy statistics and cement production data, while emissions from land-use change (ELUC), mainly deforestation, are based on combined evidence from land-cover-change data, fire activity associated with deforestation, and models. The global atmospheric CO2 concentration is measured directly and its rate of growth (GATM) is computed from the annual changes in concentration. The mean ocean CO2 sink (SOCEAN) is based on observations from the 1990s, while the annual anomalies and trends are estimated with ocean models. The variability in SOCEAN is evaluated with data products based on surveys of ocean CO2 measurements. The global residual terrestrial CO2 sink (SLAND) is estimated by the difference of the other terms of the global carbon budget and compared to results of independent dynamic global vegetation models forced by observed climate, CO2, and land-cover change (some including nitrogen–carbon interactions). We compare the mean land and ocean fluxes and their variability to estimates from three atmospheric inverse methods for three broad latitude bands. All uncertainties are reported as ±1σ, reflecting the current capacity to characterise the annual estimates of each component of the global carbon budget. For the last decade available (2005–2014), EFF was 9.0 ± 0.5 GtC yr−1, ELUC was 0.9 ± 0.5 GtC yr−1, GATM was 4.4 ± 0.1 GtC yr−1, SOCEAN was 2.6 ± 0.5 GtC yr−1, and SLAND was 3.0 ± 0.8 GtC yr−1. For the year 2014 alone, EFF grew to 9.8 ± 0.5 GtC yr−1, 0.6 % above 2013, continuing the growth trend in these emissions, albeit at a slower rate compared to the average growth of 2.2 % yr−1 that took place during 2005–2014. Also, for 2014, ELUC was 1.1 ± 0.5 GtC yr−1, GATM was 3.9 ± 0.2 GtC yr−1, SOCEAN was 2.9 ± 0.5 GtC yr−1, and SLAND was 4.1 ± 0.9 GtC yr−1. GATM was lower in 2014 compared to the past decade (2005–2014), reflecting a larger SLAND for that year. The global atmospheric CO2 concentration reached 397.15 ± 0.10 ppm averaged over 2014. For 2015, preliminary data indicate that the growth in EFF will be near or slightly below zero, with a projection of −0.6 [range of −1.6 to +0.5] %, based on national emissions projections for China and the USA, and projections of gross domestic product corrected for recent changes in the carbon intensity of the global economy for the rest of the world. From this projection of EFF and assumed constant ELUC for 2015, cumulative emissions of CO2 will reach about 555 ± 55 GtC (2035 ± 205 GtCO2) for 1870–2015, about 75 % from EFF and 25 % from ELUC. This living data update documents changes in the methods and data sets used in this new carbon budget compared with previous publications of this data set (Le Quéré et al., 2015, 2014, 2013). All observations presented here can be downloaded from the Carbon Dioxide Information Analysis Center (doi:10.3334/CDIAC/GCP_2015).