Sonnerup
Rolf E.
Sonnerup
Rolf E.
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ArticlePacific anthropogenic carbon between 1991 and 2017(American Geophysical Union, 2019-04-29) Carter, Brendan ; Feely, Richard A. ; Wanninkhof, Rik ; Kouketsu, Shinya ; Sonnerup, Rolf E. ; Pardo, Paula Conde ; Sabine, Christopher L. ; Johnson, Gregory C. ; Sloyan, Bernadette M. ; Murata, Akihiko ; Mecking, Sabine ; Tilbrook, Bronte ; Speer, Kevin G. ; Talley, Lynne D. ; Millero, Frank J. ; Wijffels, Susan E. ; Macdonald, Alison M. ; Gruber, Nicolas ; Bullister, John L.We estimate anthropogenic carbon (Canth) accumulation rates in the Pacific Ocean between 1991 and 2017 from 14 hydrographic sections that have been occupied two to four times over the past few decades, with most sections having been recently measured as part of the Global Ocean Ship‐based Hydrographic Investigations Program. The rate of change of Canth is estimated using a new method that combines the extended multiple linear regression method with improvements to address the challenges of analyzing multiple occupations of sections spaced irregularly in time. The Canth accumulation rate over the top 1,500 m of the Pacific increased from 8.8 (±1.1, 1σ) Pg of carbon per decade between 1995 and 2005 to 11.7 (±1.1) PgC per decade between 2005 and 2015. For the entire Pacific, about half of this decadal increase in the accumulation rate is attributable to the increase in atmospheric CO2, while in the South Pacific subtropical gyre this fraction is closer to one fifth. This suggests a substantial enhancement of the accumulation of Canth in the South Pacific by circulation variability and implies that a meaningful portion of the reinvigoration of the global CO2 sink that occurred between ~2000 and ~2010 could be driven by enhanced ocean Canth uptake and advection into this gyre. Our assessment suggests that the accuracy of Canth accumulation rate reconstructions along survey lines is limited by the accuracy of the full suite of hydrographic data and that a continuation of repeated surveys is a critical component of future carbon cycle monitoring.
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ArticleInfluence of mixing on CFC uptake and CFC ages in the North Pacific thermocline(American Geophysical Union, 2004-07-17) Mecking, Sabine ; Warner, Mark J. ; Greene, Catherine E. ; Hautala, Susan L. ; Sonnerup, Rolf E.A diagnostic, isopycnal advection-diffusion model based on a climatological, geostrophic flow field is used to study the uptake of chlorofluorocarbons (CFCs) into the portion of the thermocline that outcrops in the open North Pacific (σ θ ≤ 26.6 kg m−3). In addition to advection, isopycnal diffusion is required to match the CFC data collected during the World Ocean Circulation Experiment (WOCE) in the early 1990s. Using reduced outcrop saturations of 80–95% for isopycnals outcropping in the northwestern North Pacific (σ θ ≥ 25.4 kg m−3), together with an isopcynal interior diffusivity of 2000 m2 s−1 and enhanced diffusion (5000 m2 s−1) in the Kuroshio Extension region, further improves the model-data agreement. Along-isopycnal diffusion is particularly important for isopycnals with shadow zones/pool regions in the western subtropical North Pacific that are isolated from direct advective ventilation. The isopycnal mixing causes an estimated increase in CFC-12 inventories on these isopycnals, compared to advection only, ranging from 10–20% (σ θ = 25.6 kg m−3) to 50–130% (σ θ = 26.6 kg m−3) over the subtropics in 1993. This contribution has important consequences for subduction rate estimates derived from CFC inventories and for the location of the subsurface CFC maxima. When tracer ages are derived from the modeled CFC distributions, time-evolving mixing biases become apparent that reflect the nonlinearities in the atmospheric CFC time histories. Comparison with model-calculated ideal ages suggests that during the time of WOCE (∼1993), ventilation ages based on CFC-12 were biased young by as much as 16–24 years for pCFC-12 ages of 25 years, underestimating ideal ages by as much as 40–50%.