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Jong-Mi
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DatasetDissolved Pb passing through a 0.2 um Acropak capsule filter from R/V Thomas G. Thompson cruise TN303 in the Eastern Tropical Pacific in 2013 (U.S. GEOTRACES EPZT project)(Biological and Chemical Oceanography Data Management Office (BCO-DMO). Contact: bco-dmo-data@whoi.edu, 2020-09-03) Boyle, Edward A. ; Lee, Jong-Mi ; Zurbrick, CherylDissolved Pb passing through a 0.2 um Acropak capsule filter from R/V Thomas G. Thompson cruise TN303 in the Eastern Tropical Pacific in 2013. For a complete list of measurements, refer to the full dataset description in the supplemental file 'Dataset_description.pdf'. The most current version of this dataset is available at: https://www.bco-dmo.org/dataset/644607
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ArticleInsights from the U-238-th-234 method into the coupling of biological export and the cycling of cadmium, cobalt, and manganese in the southeast Pacific Ocean(American Geophysical Union, 2018-12-10) Black, Erin E. ; Lam, Phoebe J. ; Lee, Jong-Mi ; Buesseler, Kenneth O.Better constraints on the magnitude of particulate export and the residence times of trace elements are required to understand marine food web dynamics, track the transport of anthropogenic trace metals in the ocean, and improve global climate models. While prior studies have been successful in constructing basin‐scale budgets of elements like carbon in the upper ocean, the cycling of particulate trace metals is poorly understood. The 238U‐234Th method is used here with data from the GP‐16 GEOTRACES transect to investigate the upper ocean processes controlling the particulate export of cadmium, cobalt, and manganese in the southeastern Pacific. Patterns in the flux data indicated that particulate cadmium and cobalt behave similarly to particulate phosphorus and organic carbon, with the highest export in the productive coastal region and decreasing flux with depth due to remineralization. The export of manganese was influenced by redox conditions at the low oxygen coastal stations and by precipitation and/or scavenging elsewhere. Residence times with respect to export (total inventory divided by particulate flux) for phosphorus, cadmium, cobalt, and manganese in the upper 100 and 200 m were determined to be on the order of months to years. These GEOTRACES‐based synthesis efforts, combining a host of concentration and tracer data with unprecedented resolution, will help to close the oceanic budgets of trace metals.
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ArticleMajor processes of the dissolved cobalt cycle in the north and equatorial Pacific Ocean(European Geosciences Union, 2022-05-05) Chmiel, Rebecca ; Lanning, Nathan ; Laubach, Allison ; Lee, Jong-Mi ; Fitzsimmons, Jessica N. ; Hatta, Mariko ; Jenkins, William J. ; Lam, Phoebe J. ; McIlvin, Matthew R. ; Tagliabue, Alessandro ; Saito, Mak A.Over the past decade, the GEOTRACES and wider trace metal geochemical community has made substantial contributions towards constraining the marine cobalt (Co) cycle and its major biogeochemical processes. However, few Co speciation studies have been conducted in the North and equatorial Pacific Ocean, a vast portion of the world's oceans by volume and an important end-member of deep thermohaline circulation. Dissolved Co (dCo) samples, including total dissolved and labile Co, were measured at-sea during the GEOTRACES Pacific Meridional Transect (GP15) expedition along the 152∘ W longitudinal from 56∘ N to 20∘ S. Along this transect, upper-ocean dCo (σ0<26) was linearly correlated with dissolved phosphate (slope = 82±3, µmol : mol) due to phytoplankton uptake and remineralization. As depth increased, dCo concentrations became increasingly decoupled from phosphate concentrations due to co-scavenging with manganese oxide particles in the mesopelagic. The transect revealed an organically bound coastal source of dCo to the Alaskan Stream associated with low-salinity waters. An intermediate-depth hydrothermal flux of dCo was observed off the Hawaiian coast at the Loihi Seamount, and the elevated dCo was correlated with potential xs3He at and above the vent site; however, the Loihi Seamount likely did not represent a major source of Co to the Pacific basin. Elevated concentrations of dCo within oxygen minimum zones (OMZs) in the equatorial North and South Pacific were consistent with the suppression of oxidative scavenging, and we estimate that future deoxygenation could increase the OMZ dCo inventory by 18 % to 36 % over the next century. In Pacific Deep Water (PDW), a fraction of elevated ligand-bound dCo appeared protected from scavenging by the high biogenic particle flux in the North Pacific basin. This finding is counter to previous expectations of low dCo concentrations in the deep Pacific due to scavenging over thermohaline circulation. Compared to a Co global biogeochemical model, the observed transect displayed more extreme inventories and fluxes of dCo than predicted by the model, suggesting a highly dynamic Pacific Co cycle.
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PreprintThe recent distribution of lead in the Indian Ocean reflects the impact of regional emissions( 2014-09) Echegoyen, Yolanda ; Boyle, Edward A. ; Lee, Jong-Mi ; Gamo, Toshitaka ; Obata, Hajime ; Norisuye, KazuhiroHumans have injected lead (Pb) massively into the earth surface environment in a temporally and spatially evolving pattern. A significant fraction is transported by the atmosphere into the surface ocean where we can observe its transport by ocean currents and sinking particles. This study of the Indian Ocean documents high Pb concentrations in the northern and tropical surface waters, and extremely low Pb levels in the deep water. North of 20°S, dissolved Pb concentrations decrease from 42-82 pmol/Kg in surface waters to 1.5-3.3 pmol/Kg in deep waters. South of 20°S, surface water Pb concentrations decrease from 21 pmol/Kg at 31°S to 7 pmol/Kg at 62°S. This surface Pb concentration gradient reflects a southward decrease in anthropogenic Pb emissions. The upper waters of the north and central Indian Ocean have high Pb concentrations resulting from recent regional rapid industrialization and a late phase-out of leaded gasoline, and these concentrations are now higher than currently seen in the central North Pacific and North Atlantic Oceans. The Antarctic sector of the Indian Ocean shows very low concentrations due to limited regional anthropogenic Pb emissions, high scavenging rates, and rapid vertical mixing, but Pb still occurs at higher levels than would have existed centuries ago. Penetration of Pb into the northern and central Indian Ocean thermocline waters is minimized by limited ventilation. Pb concentrations in the deep Indian Ocean are comparable to the other oceans at the same latitude, and deep waters of the central Indian Ocean match the lowest observed oceanic Pb concentrations.
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ThesisEvolution of anthropogenic Pb and Pb isotopes in the deep North Atlantic Ocean and the Indian Ocean(Massachusetts Institute of Technology and Woods Hole Oceanographic Institution, 2013-06) Lee, Jong-MiPb and Pb isotopes in the ocean have varied on decadal to centennial time scales due to anthropogenic Pb inputs. Thus, tracing the temporal variation of Pb and Pb isotopes in the ocean provides information on the major sources of Pb and the transport of Pb from sources to the ocean surface and into the ocean interior. In this thesis study, first, a method was developed for the analysis of dissolved Pb and other trace elements in seawater using single batch nitrilotriacetate resin extraction and isotope dilution ICP-MS, which was applied in analyzing seawater Pb concentrations in the rest of the study. A ~550 year history of the Pb and Pb isotopes in the deep North Atlantic Ocean is reconstructed using a deep-sea coral, showing the infiltration of anthropogenic Pb to deep sea. Comparing the results to the surface North Atlantic Ocean Pb record using a Transit Time Distribution model, the mean transit time of Pb is estimated to be ~64 years. This is longer than the transit time estimate assuming simple advection from a source, showing the importance of advective-diffusive mixing in the transport of Pb to the ocean interior. The later part of the thesis investigates Pb in the Indian Ocean, where no useful Pb data have been previously reported. First, using annually-banded surface growing corals, I reconstruct variations of Pb and isotopes in the surface waters of the central and eastern Indian Oceans during the past half-century. Results of the study show the increase of Pb concentrations from the mid-1970s, and major sources of the Pb are discussed, including leaded gasoline and coal burning, based on their emission histories and Pb isotope signatures. Second, Pb concentration and isotope profiles are presented from the northern and western Indian Oceans. Higher Pb concentrations and lower Pb isotope ratios (206Pb/207Pb, 208Pb/207Pb) are found in the upper water column (<1500m) as a result of anthropogenic Pb inputs, and their distributions are largely controlled by the water circulation in the Indian Ocean.
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Working PaperEXPORTS Measurements and Protocols for the NE Pacific Campaign(NASA STI Program and Woods Hole Oceanographic Institution, 2021-02) Behrenfeld, Michael J. ; Benitez-Nelson, Claudia R. ; Boss, Emmanuel S. ; Brzezinski, Mark A. ; Buck, Kristen N. ; Buesseler, Ken O. ; Burd, Adrian B. ; Carlson, Craig A. ; Cassar, Nicolas ; Cetinić, Ivona ; Close, Hilary G. ; Craig, Susanne E. ; D'Asaro, Eric A. ; Durkin, Colleen A. ; Estapa, Margaret L. ; Fassbender, Andrea ; Fox, James ; Freeman, Scott ; Gifford, Scott M. ; Gong, Weida ; Graff, Jason R. ; Gray, Deric ; Guidi, Lionel ; Halsey, Kim ; Hansell, Dennis A. ; Haëntjens, Nils ; Horner, Tristan J. ; Jenkins, Bethany D. ; Jones, Janice L. ; Karp-Boss, Lee ; Kramer, Sasha J. ; Lam, Phoebe J. ; Lee, Craig M. ; Lee, Jong-Mi ; Liu, Shuting ; Mannino, Antonio ; Maas, Amy E. ; Marchal, Olivier ; Marchetti, Adrian ; McDonnell, Andrew M. P. ; McNair, Heather ; Menden-Deuer, Susanne ; Morison, Francoise ; Nelson, Norman B. ; Nicholson, David P. ; Niebergall, Alexandria K. ; Omand, Melissa M. ; Passow, Uta ; Perry, Mary J. ; Popp, Brian N. ; Proctor, Chris ; Rafter, Patrick ; Roca-Martí, Montserrat ; Roesler, Collin S. ; Rubin, Edwina ; Rynearson, Tatiana A. ; Santoro, Alyson E. ; Siegel, David A. ; Sosik, Heidi M. ; Soto Ramos, Inia ; Stamieszkin, Karen ; Steinberg, Deborah K. ; Stephens, Brandon M. ; Thompson, Andrew F. ; Van Mooy, Benjamin A. S. ; Zhang, XiaodongEXport Processes in the Ocean from Remote Sensing (EXPORTS) is a large-scale NASA-led and NSF co-funded field campaign that will provide critical information for quantifying the export and fate of upper ocean net primary production (NPP) using satellite information and state of the art technology.
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ArticleAn operational overview of the EXport Processes in the Ocean from RemoTe Sensing (EXPORTS) Northeast Pacific field deployment(University of California Press, 2021-07-07) Siegel, David A. ; Cetinić, Ivona ; Graff, Jason R. ; Lee, Craig M. ; Nelson, Norman B. ; Perry, Mary J. ; Soto Ramos, Inia ; Steinberg, Deborah K. ; Buesseler, Ken O. ; Hamme, Roberta C. ; Fassbender, Andrea ; Nicholson, David P. ; Omand, Melissa M. ; Robert, Marie ; Thompson, Andrew F. ; Amaral, Vinicius ; Behrenfeld, Michael J. ; Benitez-Nelson, Claudia R. ; Bisson, Kelsey ; Boss, Emmanuel S. ; Boyd, Philip ; Brzezinski, Mark A. ; Buck, Kristen N. ; Burd, Adrian B. ; Burns, Shannon ; Caprara, Salvatore ; Carlson, Craig A. ; Cassar, Nicolas ; Close, Hilary G. ; D'Asaro, Eric A. ; Durkin, Colleen A. ; Erickson, Zachary K. ; Estapa, Margaret L. ; Fields, Erik ; Fox, James ; Freeman, Scott ; Gifford, Scott M. ; Gong, Weida ; Gray, Deric ; Guidi, Lionel ; Haëntjens, Nils ; Halsey, Kim ; Huot, Yannick ; Hansell, Dennis A. ; Jenkins, Bethany D. ; Karp-Boss, Lee ; Kramer, Sasha J. ; Lam, Phoebe J. ; Lee, Jong-Mi ; Maas, Amy E. ; Marchal, Olivier ; Marchetti, Adrian ; McDonnell, Andrew M. P. ; McNair, Heather ; Menden-Deuer, Susanne ; Morison, Francoise ; Niebergall, Alexandria K. ; Passow, Uta ; Popp, Brian N. ; Potvin, Geneviève ; Resplandy, Laure ; Roca-Martí, Montserrat ; Roesler, Collin S. ; Rynearson, Tatiana A. ; Traylor, Shawnee ; Santoro, Alyson E. ; Seraphin, Kanesa ; Sosik, Heidi M. ; Stamieszkin, Karen ; Stephens, Brandon M. ; Tang, Weiyi ; Van Mooy, Benjamin ; Xiong, Yuanheng ; Zhang, XiaodongThe goal of the EXport Processes in the Ocean from RemoTe Sensing (EXPORTS) field campaign is to develop a predictive understanding of the export, fate, and carbon cycle impacts of global ocean net primary production. To accomplish this goal, observations of export flux pathways, plankton community composition, food web processes, and optical, physical, and biogeochemical (BGC) properties are needed over a range of ecosystem states. Here we introduce the first EXPORTS field deployment to Ocean Station Papa in the Northeast Pacific Ocean during summer of 2018, providing context for other papers in this special collection. The experiment was conducted with two ships: a Process Ship, focused on ecological rates, BGC fluxes, temporal changes in food web, and BGC and optical properties, that followed an instrumented Lagrangian float; and a Survey Ship that sampled BGC and optical properties in spatial patterns around the Process Ship. An array of autonomous underwater assets provided measurements over a range of spatial and temporal scales, and partnering programs and remote sensing observations provided additional observational context. The oceanographic setting was typical of late-summer conditions at Ocean Station Papa: a shallow mixed layer, strong vertical and weak horizontal gradients in hydrographic properties, sluggish sub-inertial currents, elevated macronutrient concentrations and low phytoplankton abundances. Although nutrient concentrations were consistent with previous observations, mixed layer chlorophyll was lower than typically observed, resulting in a deeper euphotic zone. Analyses of surface layer temperature and salinity found three distinct surface water types, allowing for diagnosis of whether observed changes were spatial or temporal. The 2018 EXPORTS field deployment is among the most comprehensive biological pump studies ever conducted. A second deployment to the North Atlantic Ocean occurred in spring 2021, which will be followed by focused work on data synthesis and modeling using the entire EXPORTS data set.
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ArticleThe GEOTRACES Intermediate Data Product 2017(Elsevier, 2018-06-01) Schlitzer, Reiner ; Anderson, Robert F. ; Dodas, Elena Masferrer ; Lohan, Maeve C. ; Geibert, Walter ; Tagliabue, Alessandro ; Bowie, Andrew R. ; Jeandel, Catherine ; Maldonado, Maria T. ; Landing, William M. ; Cockwell, Donna ; Abadie, Cyril ; Abouchami, Wafa ; Achterberg, Eric P. ; Agather, Alison ; Aguliar-Islas, Ana ; van Aken, Hendrik M. ; Andersen, Morten ; Archer, Corey ; Auro, Maureen E. ; Baar, Hein J. W. de ; Baars, Oliver ; Baker, Alex R. ; Bakker, Karel ; Basak, Chandranath ; Baskaran, Mark ; Bates, Nicholas R. ; Bauch, Dorothea ; van Beek, Pieter ; Behrens, Melanie K. ; Black, Erin E. ; Bluhm, Katrin ; Bopp, Laurent ; Bouman, Heather ; Bowman, Katlin ; Bown, Johann ; Boyd, Philip ; Boye, Marie ; Boyle, Edward A. ; Branellec, Pierre ; Bridgestock, Luke ; Brissebrat, Guillaume ; Browning, Thomas A. ; Bruland, Kenneth W. ; Brumsack, Hans-Jürgen ; Brzezinski, Mark A. ; Buck, Clifton S. ; Buck, Kristen N. ; Buesseler, Ken O. ; Bull, Abby ; Butler, Edward ; Cai, Pinghe ; Cámara Mor, Patricia ; Cardinal, Damien ; Carlson, Craig ; Carrasco, Gonzalo ; Casacuberta, Nuria ; Casciotti, Karen L. ; Castrillejo, Maxi ; Chamizo, Elena ; Chance, Rosie ; Charette, Matthew A. ; Chaves, Joaquin E. ; Cheng, Hai ; Chever, Fanny ; Christl, Marcus ; Church, Thomas M. ; Closset, Ivia ; Colman, Albert S. ; Conway, Tim M. ; Cossa, Daniel ; Croot, Peter L. ; Cullen, Jay T. ; Cutter, Gregory A. ; Daniels, Chris ; Dehairs, Frank ; Deng, Feifei ; Dieu, Huong Thi ; Duggan, Brian ; Dulaquais, Gabriel ; Dumousseaud, Cynthia ; Echegoyen-Sanz, Yolanda ; Edwards, R. Lawrence ; Ellwood, Michael J. ; Fahrbach, Eberhard ; Fitzsimmons, Jessica N. ; Flegal, A. Russell ; Fleisher, Martin Q. ; van de Flierdt, Tina ; Frank, Martin ; Friedrich, Jana ; Fripiat, Francois ; Fröllje, Henning ; Galer, Stephen J. G. ; Gamo, Toshitaka ; Ganeshram, Raja S. ; Garcia-Orellana, Jordi ; Garcia Solsona, Ester ; Gault-Ringold, Melanie ; George, Ejin ; Gerringa, Loes J. A. ; Gilbert, Melissa ; Godoy, Jose Marcus ; Goldstein, Steven L. ; Gonzalez, Santiago ; Grissom, Karen ; Hammerschmidt, Chad R. ; Hartman, Alison ; Hassler, Christel ; Hathorne, Ed C. ; Hatta, Mariko ; Hawco, Nicholas J. ; Hayes, Christopher T. ; Heimbürger, Lars-Eric ; Helgoe, Josh ; Heller, Maija Iris ; Henderson, Gideon M. ; Henderson, Paul B. ; van Heuven, Steven ; Ho, Peng ; Horner, Tristan J. ; Hsieh, Yu-Te ; Huang, Kuo-Fang ; Humphreys, Matthew P. ; Isshiki, Kenji ; Jacquot, Jeremy E. ; Janssen, David J. ; Jenkins, William J. ; John, Seth ; Jones, Elizabeth M. ; Jones, Janice L. ; Kadko, David ; Kayser, Rick ; Kenna, Timothy C. ; Khondoker, Roulin ; Kim, Taejin ; Kipp, Lauren ; Klar, Jessica K. ; Klunder, Maarten ; Kretschmer, Sven ; Kumamoto, Yuichiro ; Laan, Patrick ; Labatut, Marie ; Lacan, Francois ; Lam, Phoebe J. ; Lambelet, Myriam ; Lamborg, Carl H. ; le Moigne, Frederique ; Le Roy, Emilie ; Lechtenfeld, Oliver J. ; Lee, Jong-Mi ; Lherminier, Pascale ; Little, Susan ; López-Lora, Mercedes ; Lu, Yanbin ; Masque, Pere ; Mawji, Edward ; McClain, Charles R. ; Measures, Christopher I. ; Mehic, Sanjin ; Menzel Barraqueta, Jan-Lukas ; Merwe, Pier van der ; Middag, Rob ; Mieruch, Sebastian ; Milne, Angela ; Minami, Tomoharu ; Moffett, James W. ; Moncoiffe, Gwenaelle ; Moore, Willard S. ; Morris, Paul J. ; Morton, Peter L. ; Nakaguchi, Yuzuru ; Nakayama, Noriko ; Niedermiller, John ; Nishioka, Jun ; Nishiuchi, Akira ; Noble, Abigail E. ; Obata, Hajime ; Ober, Sven ; Ohnemus, Daniel C. ; van Ooijen, Jan ; O'Sullivan, Jeanette ; Owens, Stephanie A. ; Pahnke, Katharina ; Paul, Maxence ; Pavia, Frank ; Pena, Leopoldo D. ; Peters, Brian ; Planchon, Frederic ; Planquette, Helene ; Pradoux, Catherine ; Puigcorbé, Viena ; Quay, Paul D. ; Queroue, Fabien ; Radic, Amandine ; Rauschenberg, Sara ; Rehkämper, Mark ; Rember, Robert ; Remenyi, Tomas A. ; Resing, Joseph A. ; Rickli, Joerg ; Rigaud, Sylvain ; Rijkenberg, Micha J. A. ; Rintoul, Stephen R. ; Robinson, Laura F. ; Roca-Martí, Montserrat ; Rodellas, Valenti ; Roeske, Tobias ; Rolison, John M. ; Rosenberg, Mark ; Roshan, Saeed ; Rutgers van der Loeff, Michiel M. ; Ryabenko, Evgenia ; Saito, Mak A. ; Salt, Lesley ; Sanial, Virginie ; Sarthou, Geraldine ; Schallenberg, Christina ; Schauer, Ursula ; Scher, Howie ; Schlosser, Christian ; Schnetger, Bernhard ; Scott, Peter M. ; Sedwick, Peter N. ; Semiletov, Igor P. ; Shelley, Rachel U. ; Sherrell, Robert M. ; Shiller, Alan M. ; Sigman, Daniel M. ; Singh, Sunil Kumar ; Slagter, Hans ; Slater, Emma ; Smethie, William M. ; Snaith, Helen ; Sohrin, Yoshiki ; Sohst, Bettina M. ; Sonke, Jeroen E. ; Speich, Sabrina ; Steinfeldt, Reiner ; Stewart, Gillian ; Stichel, Torben ; Stirling, Claudine H. ; Stutsman, Johnny ; Swarr, Gretchen J. ; Swift, James H. ; Thomas, Alexander ; Thorne, Kay ; Till, Claire P. ; Till, Ralph ; Townsend, Ashley T. ; Townsend, Emily ; Tuerena, Robyn ; Twining, Benjamin S. ; Vance, Derek ; Velazquez, Sue ; Venchiarutti, Celia ; Villa-Alfageme, Maria ; Vivancos, Sebastian M. ; Voelker, Antje H. L. ; Wake, Bronwyn ; Warner, Mark J. ; Watson, Ros ; van Weerlee, Evaline ; Weigand, M. Alexandra ; Weinstein, Yishai ; Weiss, Dominik ; Wisotzki, Andreas ; Woodward, E. Malcolm S. ; Wu, Jingfeng ; Wu, Yingzhe ; Wuttig, Kathrin ; Wyatt, Neil ; Xiang, Yang ; Xie, Ruifang C. ; Xue, Zichen ; Yoshikawa, Hisayuki ; Zhang, Jing ; Zhang, Pu ; Zhao, Ye ; Zheng, Linjie ; Zheng, Xin-Yuan ; Zieringer, Moritz ; Zimmer, Louise A. ; Ziveri, Patrizia ; Zunino, Patricia ; Zurbrick, CherylThe GEOTRACES Intermediate Data Product 2017 (IDP2017) is the second publicly available data product of the international GEOTRACES programme, and contains data measured and quality controlled before the end of 2016. The IDP2017 includes data from the Atlantic, Pacific, Arctic, Southern and Indian oceans, with about twice the data volume of the previous IDP2014. For the first time, the IDP2017 contains data for a large suite of biogeochemical parameters as well as aerosol and rain data characterising atmospheric trace element and isotope (TEI) sources. The TEI data in the IDP2017 are quality controlled by careful assessment of intercalibration results and multi-laboratory data comparisons at crossover stations. The IDP2017 consists of two parts: (1) a compilation of digital data for more than 450 TEIs as well as standard hydrographic parameters, and (2) the eGEOTRACES Electronic Atlas providing an on-line atlas that includes more than 590 section plots and 130 animated 3D scenes. The digital data are provided in several formats, including ASCII, Excel spreadsheet, netCDF, and Ocean Data View collection. Users can download the full data packages or make their own custom selections with a new on-line data extraction service. In addition to the actual data values, the IDP2017 also contains data quality flags and 1-σ data error values where available. Quality flags and error values are useful for data filtering and for statistical analysis. Metadata about data originators, analytical methods and original publications related to the data are linked in an easily accessible way. The eGEOTRACES Electronic Atlas is the visual representation of the IDP2017 as section plots and rotating 3D scenes. The basin-wide 3D scenes combine data from many cruises and provide quick overviews of large-scale tracer distributions. These 3D scenes provide geographical and bathymetric context that is crucial for the interpretation and assessment of tracer plumes near ocean margins or along ridges. The IDP2017 is the result of a truly international effort involving 326 researchers from 25 countries. This publication provides the critical reference for unpublished data, as well as for studies that make use of a large cross-section of data from the IDP2017. This article is part of a special issue entitled: Conway GEOTRACES - edited by Tim M. Conway, Tristan Horner, Yves Plancherel, and Aridane G. González.