Wozniak Andrew S.

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Wozniak
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Andrew S.
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  • Working Paper
    US SOLAS Science Report
    (Woods Hole Oceanographic Institution, 2021-12) Stanley, Rachel H. R. ; Bell, Tom G. ; Gao, Yuan ; Gaston, Cassandra J. ; Ho, David T. ; Kieber, David J. ; Mackey, Katherine R. M. ; Meskhidze, Nicholas ; Miller, William L. ; Potter, Henry ; Vlahos, Penny ; Yager, Patricia L. ; Alexander, Becky ; Beaupre, Steven R. ; Craig, Susanne E. ; Cutter, Gregory A. ; Emerson, Steven ; Frossard, Amanda A. ; Gasso, Santiago ; Haus, Brian K. ; Keene, William C. ; Landing, William M. ; Moore, Richard H. ; Ortiz-Suslow, David ; Palter, Jaime B. ; Paulot, Fabien ; Saltzman, Eric ; Thornton, Daniel ; Wozniak, Andrew S. ; Zamora, Lauren M. ; Benway, Heather M.
    The Surface Ocean – Lower Atmosphere Study (SOLAS) (http://www.solas-int.org/) is an international research initiative focused on understanding the key biogeochemical-physical interactions and feedbacks between the ocean and atmosphere that are critical elements of climate and global biogeochemical cycles. Following the release of the SOLAS Decadal Science Plan (2015-2025) (Brévière et al., 2016), the Ocean-Atmosphere Interaction Committee (OAIC) was formed as a subcommittee of the Ocean Carbon and Biogeochemistry (OCB) Scientific Steering Committee to coordinate US SOLAS efforts and activities, facilitate interactions among atmospheric and ocean scientists, and strengthen US contributions to international SOLAS. In October 2019, with support from OCB, the OAIC convened an open community workshop, Ocean-Atmosphere Interactions: Scoping directions for new research with the goal of fostering new collaborations and identifying knowledge gaps and high-priority science questions to formulate a US SOLAS Science Plan. Based on presentations and discussions at the workshop, the OAIC and workshop participants have developed this US SOLAS Science Plan. The first part of the workshop and this Science Plan were purposefully designed around the five themes of the SOLAS Decadal Science Plan (2015-2025) (Brévière et al., 2016) to provide a common set of research priorities and ensure a more cohesive US contribution to international SOLAS.
  • Article
    Isotopic characterization of aerosol organic carbon components over the eastern United States
    (American Geophysical Union, 2012-07-04) Wozniak, Andrew S. ; Bauer, James E. ; Dickhut, Rebecca M. ; Xu, Li ; McNichol, Ann P.
    Carbon isotopic signatures (δ13C, Δ14C) of aerosol particulate matter total organic carbon (TOC) and operationally defined organic carbon (OC) components were measured in samples from two background sites in the eastern U.S. TOC and water-soluble OC (WSOC) δ13C values (−27 to −24‰) indicated predominantly terrestrial C3 plant and fossil derived sources. Total solvent extracts (TSE) and their aliphatic, aromatic, and polar OC components were depleted in δ13C (−30 to −26‰) relative to TOC and WSOC. Δ14C signatures of aerosol TOC and TSE (−476 to +25‰) suggest variable fossil contributions (~5–50%) to these components. Aliphatic OC while comprising a small portion of the TOC (<1%), was dominated by fossil-derived carbon (86 ± 3%), indicating its potential utility as a tracer for fossil aerosol OC inputs. In contrast, aromatic OC contributions (<1.5%) contained approximately equal portions contemporary (52 ± 8%) and fossil (48 ± 8%) OC. The quantitatively significant polar OC fraction (6–25% of TOC) had fossil contributions (30 ± 12%) similar to TOC (26 ± 7%) and TSE (28 ± 9%). Thus, much of both of the fossil and contemporary OC is deduced to be oxidized, polar material. Aerosol WSOC consistently showed low fossil content (<8%) relative to the TOC (5–50%) indicating that the majority of fossil OC in aerosol particulates is insoluble. Therefore, on the basis of solubility and polarity, aerosols are predicted to partition differently once deposited to watersheds, and these chemically distinct components are predicted to contribute in quantitatively and qualitatively different ways to watershed carbon biogeochemistry and cycling.
  • Article
    Correction to “Isotopic characterization of aerosol organic carbon components over the eastern United States”
    (American Geophysical Union, 2012-08-02) Wozniak, Andrew S. ; Bauer, James E. ; Dickhut, Rebecca M. ; Xu, Li ; McNichol, Ann P.
  • Article
    Identification of next-generation International Humic Substances Society reference materials for advancing the understanding of the role of natural organic matter in the Anthropocene
    (Springer, 2023-01-09) Chin, Yu-Ping ; McKnight, Diane M. ; D’Andrilli, Juliana ; Brooks, Nicole ; Cawley, Kaelin ; Guerard, Jennifer ; Perdue, E. Michael ; Stedmon, Colin A. ; Tratnyek, Paul G. ; Westerhoff, Paul ; Wozniak, Andrew S. ; Bloom, Paul R. ; Foreman, Christine M. ; Gabor, Rachel ; Hamdi, Jumanah ; Hanson, Blair ; Hozalski, Raymond M. ; Kellerman, Anne M. ; McKay, Garrett ; Silverman, Victoria ; Spencer, Robert G. M. ; Ward, Collin P. ; Xin, Danhui ; Rosario-Ortiz, Fernando ; Remucal, Christina K. ; Reckhow, David
    Many challenges remain before we can fully understand the multifaceted role that natural organic matter (NOM) plays in soil and aquatic systems. These challenges remain despite the considerable progress that has been made in understanding NOM’s properties and reactivity using the latest analytical techniques. For nearly 4 decades, the International Humic Substances Society (IHSS, which is a non-profit scientific society) has distributed standard substances that adhere to strict isolation protocols and reference materials that are collected in bulk and originate from clearly defined sites. These NOM standard and reference samples offer relatively uniform materials for designing experiments and developing new analytical methods. The protocols for isolating NOM, and humic and fulvic acid fractions of NOM utilize well-established preparative scale column chromatography and reverse osmosis methods. These standard and reference NOM samples are used by the international scientific community to study NOM across a range of disciplines from engineered to natural systems, thereby seeding the transfer of knowledge across research fields. Recently, powerful new analytical techniques used to characterize NOM have revealed complexities in its composition that transcend the “microbial” vs. “terrestrial” precursor paradigm. To continue to advance NOM research in the Anthropocene epoch, a workshop was convened to identify potential new sites for NOM samples that would encompass a range of sources and precursor materials and would be relevant for studying NOM’s role in mediating environmental and biogeochemical processes. We anticipate that expanding the portfolio of IHSS reference and standard NOM samples available to the research community will enable this diverse group of scientists and engineers to better understand the role that NOM plays globally under the influence of anthropogenic mediated changes.