Wagner Thomas

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Wagner
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Thomas
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  • Article
    Organic matter in river-influenced continental margin sediments : the land-ocean and climate linkage at the Late Quaternary Congo fan (ODP Site 1075)
    (American Geophysical Union, 2003-12-31) Holtvoeth, Jens ; Wagner, Thomas ; Schubert, Carsten J.
    Late Quaternary sections (1.2 Ma) of ODP-Site 1075 from the Congo deep-sea fan are investigated to reconstruct variations of terrigenous organic matter supply to the eastern equatorial Atlantic. To characterize the organic matter (OM) with regard to marine and terrigenous amounts we used elemental analysis (C, N, S), stable carbon isotopes (bulk δ13Corg), Rock-Eval pyrolysis, and terrigenous biomarkers (lignin phenols from CuO oxidation). The records of total organic carbon (TOC) contents, Corg/Ntot ratios, bulk OM degradation rates (Corg/Corg*), and the ratios of hydrocarbons (HC) from low-mature versus HC from high-mature OM (lm/hm) reveal pronounced cyclic changes in OM abundance, preservation, and reactivity that are closely related to the precessional controlled record of insolation, and thus, to variations in upwelling intensity and fluvial run-off. Primary productivity off the Congo is stimulated by both, enhanced nutrient supply in response to trade-induced upwelling during arid African climates (insolation minima) and fluvial nutrient delivery during humid stages (following insolation maxima), especially due to the contribution of dissolved silica that is taken up preferably by diatoms. However, results stemming from a multiparameter approach reveal that the fluvial supply of degraded OM and black carbon (BC) associated with fine-grained sediments from soil erosion is a decisive factor for the preservation of marine OM and, in addition, significantly influences the geochemical signature of bulk and terrigenous OM. Riverine and eolian supply of C4 plant matter, as well as enhanced concentrations of BC, during arid and arid-to-humid transitional climate stages, may lead to a severe underestimation of terrigenous organic carbon, if its amount is calculated from bulk isotopic ratios using binary end-member models. During the humid stages, it is the massive supply of 13C-enriched soil OM with low Corg/Ntot ratios that may suggest a mainly marine composition of bulk OM. In fact, terrigenous OM governs bulk OM geochemical signatures in the sediments of the Congo deep-sea fan, a result that is contradictory to earlier studies, especially to the conventional interpretation of the bulk δ13Corg signal.
  • Article
    Rapid analysis of 13C in plant-wax n-alkanes for reconstruction of terrestrial vegetation signals from aquatic sediments
    (American Geophysical Union, 2004-10-15) McDuffee, Kelsey E. ; Eglinton, Timothy I. ; Sessions, Alex L. ; Sylva, Sean P. ; Wagner, Thomas ; Hayes, John M.
    Long-chain, odd-carbon-numbered C25 to C35 n-alkanes are characteristic components of epicuticular waxes produced by terrestrial higher plants. They are delivered to aquatic systems via eolian and fluvial transport and are preserved in underlying sediments. The isotopic compositions of these products can serve as records of past vegetation. We have developed a rapid method for stable carbon isotopic analyses of total plant-wax n-alkanes using a novel, moving-wire system coupled to an isotope-ratio mass spectrometer (MW-irMS). The n-alkane fractions are prepared from sediment samples by (1) saponification and extraction with organic solvents, (2) chromatographic separation using silica gel, (3) isolation of straight-chain carbon skeletons using a zeolite molecular sieve, and (4) oxidation and removal of unsaturated hydrocarbons with RuO4. Short-chain n-alkanes of nonvascular plant origin (
  • Article
    EUREC4A
    (Copernicus Publications, 2021-08-25) Stevens, Bjorn ; Bony, Sandrine ; Farrell, David ; Ament, Felix ; Blyth, Alan ; Fairall, Christopher W. ; Karstensen, Johannes ; Quinn, Patricia K. ; Speich, Sabrina ; Acquistapace, Claudia ; Aemisegger, Franziska ; Albright, Anna Lea ; Bellenger, Hugo ; Bodenschatz, Eberhard ; Caesar, Kathy-Ann ; Chewitt-Lucas, Rebecca ; de Boer, Gijs ; Delanoë, Julien ; Denby, Leif ; Ewald, Florian ; Fildier, Benjamin ; Forde, Marvin ; George, Geet ; Gross, Silke ; Hagen, Martin ; Hausold, Andrea ; Heywood, Karen J. ; Hirsch, Lutz ; Jacob, Marek ; Jansen, Friedhelm ; Kinne, Stefan ; Klocke, Daniel ; Kölling, Tobias ; Konow, Heike ; Lothon, Marie ; Mohr, Wiebke ; Naumann, Ann Kristin ; Nuijens, Louise ; Olivier, Léa ; Pincus, Robert ; Pöhlker, Mira L. ; Reverdin, Gilles ; Roberts, Gregory ; Schnitt, Sabrina ; Schulz, Hauke ; Siebesma, Pier ; Stephan, Claudia Christine ; Sullivan, Peter P. ; Touzé-Peiffer, Ludovic ; Vial, Jessica ; Vogel, Raphaela ; Zuidema, Paquita ; Alexander, Nicola ; Alves, Lyndon ; Arixi, Sophian ; Asmath, Hamish ; Bagheri, Gholamhossein ; Baier, Katharina ; Bailey, Adriana ; Baranowski, Dariusz ; Baron, Alexandre ; Barrau, Sébastien ; Barrett, Paul A. ; Batier, Frédéric ; Behrendt, Andreas ; Bendinger, Arne ; Beucher, Florent ; Bigorre, Sebastien P. ; Blades, Edmund ; Blossey, Peter ; Bock, Olivier ; Böing, Steven ; Bosser, Pierre ; Bourras, Denis ; Bouruet-Aubertot, Pascale ; Bower, Keith ; Branellec, Pierre ; Branger, Hubert ; Brennek, Michal ; Brewer, Alan ; Brilouet, Pierre-Etienne ; Brügmann, Björn ; Buehler, Stefan A. ; Burke, Elmo ; Burton, Ralph ; Calmer, Radiance ; Canonici, Jean-Christophe ; Carton, Xavier ; Cato, Gregory, Jr. ; Charles, Jude Andre ; Chazette, Patrick ; Chen, Yanxu ; Chilinski, Michal T. ; Choularton, Thomas ; Chuang, Patrick ; Clarke, Shamal ; Coe, Hugh ; Cornet, Céline ; Coutris, Pierre ; Couvreux, Fleur ; Crewell, Susanne ; Cronin, Timothy W. ; Cui, Zhiqiang ; Cuypers, Yannis ; Daley, Alton ; Damerell, Gillian M. ; Dauhut, Thibaut ; Deneke, Hartwig ; Desbios, Jean-Philippe ; Dörner, Steffen ; Donner, Sebastian ; Douet, Vincent ; Drushka, Kyla ; Dütsch, Marina ; Ehrlich, André ; Emanuel, Kerry A. ; Emmanouilidis, Alexandros ; Etienne, Jean-Claude ; Etienne-Leblanc, Sheryl ; Faure, Ghislain ; Feingold, Graham ; Ferrero, Luca ; Fix, Andreas ; Flamant, Cyrille ; Flatau, Piotr Jacek ; Foltz, Gregory R. ; Forster, Linda ; Furtuna, Iulian ; Gadian, Alan ; Galewsky, Joseph ; Gallagher, Martin ; Gallimore, Peter ; Gaston, Cassandra J. ; Gentemann, Chelle L. ; Geyskens, Nicolas ; Giez, Andreas ; Gollop, John ; Gouirand, Isabelle ; Gourbeyre, Christophe ; de Graaf, Dörte ; de Graaf, Geiske E. ; Grosz, Robert ; Güttler, Johannes ; Gutleben, Manuel ; Hall, Kashawn ; Harris, George ; Helfer, Kevin C. ; Henze, Dean ; Herbert, Calvert ; Holanda, Bruna ; Ibanez-Landeta, Antonio ; Intrieri, Janet ; Iyer, Suneil ; Julien, Fabrice ; Kalesse, Heike ; Kazil, Jan ; Kellman, Alexander ; Kidane, Abiel T. ; Kirchner, Ulrike ; Klingebiel, Marcus ; Körner, Mareike ; Kremper, Leslie Ann ; Kretzschmar, Jan ; Krüger, Ovid O. ; Kumala, Wojciech ; Kurz, Armin ; L'Hégareta, Pierre ; Labaste, Matthieu ; Lachlan-Cope, Thomas ; Laing, Arlene ; Landschützer, Peter ; Lang, Theresa ; Lange, Diego ; Lange, Ingo ; Laplace, Clément ; Lavik, Gauke ; Laxenaire, Rémi ; Le Bihan, Caroline ; Leandro, Mason ; Lefevre, Nathalie ; Lena, Marius ; Lenschow, Donald ; Li, Qiang ; Lloyd, Gary ; Los, Sebastian ; Losi, Niccolò ; Lovell, Oscar ; Luneau, Christopher ; Makuch, Przemyslaw ; Malinowski, Szymon ; Manta, Gaston ; Marinou, Eleni ; Marsden, Nicholas ; Masson, Sebastien ; Maury, Nicolas ; Mayer, Bernhard ; Mayers-Als, Margarette ; Mazel, Christophe ; McGeary, Wayne ; McWilliams, James C. ; Mech, Mario ; Mehlmann, Melina ; Meroni, Agostino Niyonkuru ; Mieslinger, Theresa ; Minikin, Andreas ; Minnett, Peter J. ; Möller, Gregor ; Morfa Avalos, Yanmichel ; Muller, Caroline ; Musat, Ionela ; Napoli, Anna ; Neuberger, Almuth ; Noisel, Christophe ; Noone, David ; Nordsiek, Freja ; Nowak, Jakub L. ; Oswald, Lothar ; Parker, Douglas J. ; Peck, Carolyn ; Person, Renaud ; Philippi, Miriam ; Plueddemann, Albert J. ; Pöhlker, Christopher ; Pörtge, Veronika ; Pöschl, Ulrich ; Pologne, Lawrence ; Posyniak, Michał ; Prange, Marc ; Quinones Melendez, Estefania ; Radtke, Jule ; Ramage, Karim ; Reimann, Jens ; Renault, Lionel ; Reus, Klaus ; Reyes, Ashford ; Ribbe, Joachim ; Ringel, Maximilian ; Ritschel, Markus ; Rocha, Cesar B. ; Rochetin, Nicolas ; Röttenbacher, Johannes ; Rollo, Callum ; Royer, Haley M. ; Sadoulet, Pauline ; Saffin, Leo ; Sandiford, Sanola ; Sandu, Irina ; Schäfer, Michael ; Schemann, Vera ; Schirmacher, Imke ; Schlenczek, Oliver ; Schmidt, Jerome M. ; Schröder, Marcel ; Schwarzenboeck, Alfons ; Sealy, Andrea ; Senff, Christoph J. ; Serikov, Ilya ; Shohan, Samkeyat ; Siddle, Elizabeth ; Smirnov, Alexander ; Späth, Florian ; Spooner, Branden ; Stolla, M. Katharina ; Szkółka, Wojciech ; de Szoeke, Simon P. ; Tarot, Stéphane ; Tetoni, Eleni ; Thompson, Elizabeth ; Thomson, Jim ; Tomassini, Lorenzo ; Totems, Julien ; Ubele, Alma Anna ; Villiger, Leonie ; von Arx, Jan ; Wagner, Thomas ; Walther, Andi ; Webber, Ben ; Wendisch, Manfred ; Whitehall, Shanice ; Wiltshire, Anton ; Wing, Allison A. ; Wirth, Martin ; Wiskandt, Jonathan ; Wolf, Kevin ; Worbes, Ludwig ; Wright, Ethan ; Young, Shanea ; Zhang, Chidong ; Zhang, Dongxiao ; Ziemen, Florian ; Zinner, Tobias ; Zöger, Martin
    The science guiding the EUREC4A campaign and its measurements is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. Through its ability to characterize processes operating across a wide range of scales, EUREC4A marked a turning point in our ability to observationally study factors influencing clouds in the trades, how they will respond to warming, and their link to other components of the earth system, such as upper-ocean processes or the life cycle of particulate matter. This characterization was made possible by thousands (2500) of sondes distributed to measure circulations on meso- (200 km) and larger (500 km) scales, roughly 400 h of flight time by four heavily instrumented research aircraft; four global-class research vessels; an advanced ground-based cloud observatory; scores of autonomous observing platforms operating in the upper ocean (nearly 10 000 profiles), lower atmosphere (continuous profiling), and along the air–sea interface; a network of water stable isotopologue measurements; targeted tasking of satellite remote sensing; and modeling with a new generation of weather and climate models. In addition to providing an outline of the novel measurements and their composition into a unified and coordinated campaign, the six distinct scientific facets that EUREC4A explored – from North Brazil Current rings to turbulence-induced clustering of cloud droplets and its influence on warm-rain formation – are presented along with an overview of EUREC4A's outreach activities, environmental impact, and guidelines for scientific practice. Track data for all platforms are standardized and accessible at https://doi.org/10.25326/165 (Stevens, 2021), and a film documenting the campaign is provided as a video supplement.
  • Article
    Unraveling Environmental Forces Shaping Surface Sediment Geochemical “Isodrapes” in the East Asian Marginal Seas
    (American Geophysical Union, 2024-04-04) Paradis, Sarah ; Diesing, Markus ; Gies, Hannah ; Haghipour, Negar ; Narman, Lena ; Magill, Clayton ; Wagner, Thomas ; Galy, Valier V. ; Hou, Pengfei ; Zhao, Meixun ; Kim, Jung-Hyun ; Shin, Kyung-Hoon ; Lin, Baozhi ; Liu, Zhifei ; Wiesner, Martin G. ; Stattegger, Karl ; Chen, Jianfang ; Zhang, Jingjing ; Eglinton, Timothy I.
    As major sites of carbon burial and remineralization, continental margins are key components of the global carbon cycle. However, heterogeneous sources of organic matter (OM) and depositional environments lead to complex spatial patterns in sedimentary organic carbon (OC) content and composition. To better constrain the processes that control OM cycling, we focus on the East Asian marginal seas as a model system, where we compiled extensive data on the OC content, bulk isotopic composition (δ13C and Δ14C), total nitrogen, and mineral surface area of surficial sediments from previous studies and new measurements. We developed a spatial machine learning modeling framework to predict the spatial distribution of these parameters and identify regions where sediments with similar geochemical signatures drape the seafloor (i.e., “isodrapes”). We demonstrate that both provenance (44%–77%) and hydrodynamic processes (22%–53%) govern the fate of OM in this margin. Hydrodynamic processes can either promote the degradation of OM in mobile mud-belts or preserve it in stable mud-deposits. The distinct isotopic composition of OC sources from marine productivity and individual rivers regulates the age and reactivity of OM deposited on the sea-floor. The East Asian marginal seas can be separated into three main isodrapes: hydrodynamically energetic shelves with coarser-grained sediment depleted in OC, OM-enriched mud deposits, and a deep basin with fine-grained sediments and aged OC affected by long oxygen exposure times and petrogenic input from rivers. This study confirms that both hydrodynamic processes and provenance should be accounted for to understand the fate of OC in continental margins.